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MOSI纳米线的非平衡光学特性

Non-equilibrium optical properties of MoSI nanowires
课程网址: http://videolectures.net/slonano07_gagermaier_nop/  
主讲教师: Christoph Gadermaier
开课单位: 约瑟夫·斯特凡学院
开课时间: 2008-02-12
课程语种: 英语
中文简介:
MoSI纳米线是一维系统,与邻居之间的相互作用最弱。因此,他们应该最清楚地表明一维性的影响。我们通过光学反射率和吸光度以及定向Mo6S3I6纳米线薄膜的飞秒泵浦 - 探针光谱研究了平衡和非平衡光学性质。平行于取向轴偏振的光的吸收显示出一系列垂直偏振不存在的共振。没有观察到材料的高度一维特征所预期的尖锐的Van Hove特征,部分原因是电子子带的密度大,部分是因为电子能量阻尼。通过飞秒泵浦探针光谱研究了非平衡情况下的电子弛豫。通过激发第二个光学共振,我们发现了涉及三种不同激发态的复杂弛豫行为,并确定了所涉及状态的寿命。
课程简介: MoSI nanowires are the one-dimensional systems with the weakest known interaction with their neighbours. Therefore they are expected to show most clearly the effects of one-dimensionality. We studied equilibrium and non-equilibrium optical properties via optical reflectivity and absorbance as well as femtosecond pump-probe spectra of oriented Mo6S3I6 nanowire thin films. Absorption of light polarised parallel to the axis of orientation shows a series of resonances that are absent for perpendicular polarisation. The sharp Van Hove features expected from the highly one-dimensional character of the material are not observed, partly because of the large density of electron sub-bands and partly because of electron energy damping. The electronic relaxation from a non-equilibrium situation was studied via femtosecond pump-probe spectroscopy. By exciting into the second optical resonance we found a complex relaxation behaviour involving three distinct excited states and determined the lifetimes of the involved states.
关 键 词: 莫思纳米线; 第二光学谐振; 光学反射率
课程来源: 视频讲座网
最后编审: 2020-07-29:yumf
阅读次数: 66